Isotopes of uranium in the waters of mine tailings Kadzhi-Sai
Abstract
The paper presents the results of the determination of uranium isotopes in the water objects of the region Kadzhi-Sai, where former uranium mine, concentrating plant and tailing with a total volume of 400,000 m3 are located. Determination of uranium isotopes was done by alpha-spectrometry method with previous radiochemical preparation (coprecipitation on iron hydroxide, extraction with tributyl phosphate and electrodeposition on stainless steel disk) on alpha-spectrometer of «Canberra». On the basis of experimental data, the ratios of uranium-234 to uranium-238 were calculated, uranium isotope chart of determination of genetic composition of water were built and investigated. During the work three genetic types of waters were established: waters of deep circulation, waters of uranium anomalies draining tailing, and waters of active water exchange of the region. Their mixing proportions in the investigated water sources were calculated. It was found that drinking waters of Kadzhi-Sai village consist of only 5-7% of waters enriched by uranium; the major part (60-80%) is waters of deep circulation.
References
1 (1970-1981) Great Soviet Encyclopedia [Bolshaya Sovetskaya Encyclopedia]. Sovetskaya Encyclopedia, Moscow, Russia. 30 volumes. (In Russian)
2 Matychenkov VE, Tynybekov AK (2000) Hydrochemical and ecological characteristics of the composition of the water of the rivers of Southern Issyk-Kul region [Gidrohimicheskaja i jekologicheskaja harakteristika sostava vody rek Juzhnogo Priissykkul’ja]. Abstracts of Kyrgyz Institute of mineral raw materials, Bishkek, Kyrgyzstan. P.101-110. (In Russian)
3 Samsonova AA, Zubkov EB, Mambetaliyev EDj (2005) The results of regime observations of uranium content in groundwater in the valley Djilu-Bulak [Rezul’taty rezhimnyh nabljudenij za soderzhaniem urana v podzemnyh vodah v doline Dzhilu-Bulak]. Chapter in: The study of the hydrodynamics of Issyk-Kul Lake with the usage of isotope techniques, Ilim, Bishkek, Kyrgyzstan. Part I. P.152-159. (In Russian)
4 Samsonova AA, Zubkov EB, Mambetaliev EDj, Matychenkova MV (2006) Uranium Content in Underground Waters of Djilu-Bulak Valley. Chapter in: Study of the Issik-Kul Lake Hydrodynamics with the Use of Isotopic Methods. Ilim, Bishkek, Kyrgyzstan. Part II. P.116-123.
5 Romanovsky V, Mamatkanov D et al. (2014) All about Issyk-Kul Lake [Vse ob ozere Issyk-Kul’]. Chapter in: Encyclopedic Handbook of the lake and basin in questions and answers, IVPiGJe NAN KR, Bishkek, Kyrgyzstan. P.162-164. (In Russian)
6 (1999) 381–NPh. Methods of measurement of volume activity of uranium isotopes (234, 238) in natural water samples by alpha spectrometry with radiochemical separation [381–JaF Metodika vypolnenija izmerenij ob`emnoj aktivnosti izotopov urana (234, 238) v probah prirodnyh vod al’fa-spektrometricheskim metodom s radiohimicheskim vydeleniem]. Moscow, Russia. (In Russian)
7 Uralbekov BM, Burkitbayev ММ, Mamatkanov D, Matveyeva IV, Satybaldyev BS, Tuzova TV (2013) Uranium isotopes in the waters of Chu basin [Izotopy urana v vodah bassejna r.Chu]. Materials of the 4th International Conference “Radioactivity and radioactive elements in the human environment”, Tomsk, Russia. P.535-537. (In Russian)
8 Uralbekov B, Burkitbaev M, Satybaldiev B, Matveyeva I, Tuzova T, Snow D (2014) Environmental Earth Sciences 4:148-155. http://dx.doi.org/10.1007/s12665-014-3274-x
9 Chalov PI, Vasiliev IA, Tolstikhin GM et al (2000) The content, isotopic composition and spatial distribution of the main radioactive uranium series in groundwater areas of Kara-Balta [Soderzhanie, izotopnyj sostav i prostranstvennoe raspredelenie osnovnyh radiojelementov uranovogo rjada v podzemnyh vodah Kara-Baltinskoj ploshhadi]. Chapter in: Radiological and associated problems of uranium production. Ilim, Bishkek, Kyrgyzstan. P.36-47. (In Russian)
10 Burkitbayev MM, Uralbekov BM, Stegnar P, Shishkov IA, Matveyeva IV (2007) Chemical Journal of Kazakhstan [Himicheskij zhurnal Kazahstana] 3:44-78. (In Russian)
11 Uralbekov B, Smodiš B and Burkitbayev M (2011) Journal of Radioanalytical and Nuclear Chemistry 289(3):805-810. http://dx.doi.org/10.1007/s10967-011-1154-3
12 Burkitbayev M, Uralbekov B, Nazarkulova Sh, Matveyeva I, León LV (2012) Journal of Environmental Monitoring 14:1190-1195. http://dx.doi.org/10.1039/c2em11014h
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